Advances in Electrochemical Science and Engineering, Volume by Richard C. Alkire, Charles W. Tobias PDF

By Richard C. Alkire, Charles W. Tobias

ISBN-10: 352729385X

ISBN-13: 9783527293858

ISBN-10: 3527616799

ISBN-13: 9783527616794

ISBN-10: 3527616888

ISBN-13: 9783527616886

This sequence, previously edited by means of Heinz Gerischer and Charls V. Tobias, now edited by way of Richard C. Alkire and Dieter M. Kolb, has been warmly welcomed via scientists world-wide that is mirrored within the experiences of the former volumes:

'This is an important ebook for researchers in electrochemistry; it covers components of either primary and sensible value, with studies of top of the range. the fabric is especially good offered and the alternative of subject matters displays a balanced editorial coverage that's welcomed.' The Analyst

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Additional info for Advances in Electrochemical Science and Engineering, Volume 5

Sample text

1 Aromatic Hydrocarbons Aromatic hydrocarbons, with the reaction scheme as described above, play the same key role in ECL studies as in organic electrochemistry and organic UV-VIS spectroscopy. 5,6,11,12-Tetraphenyltetracene(rubrene) and 9,lO-diphenylanthracene (DPA) are the most notable examples (Fig. 10). The stability of their radical ions, with the quantum efficiency q50 of the parent molecules near unity, [121] has fascinated many ECL investigators since the 1960s ([122,123] and cited references).

The quantities needed (Air&,, and V3) are chosen to obtain the best fit between experimentally found and theoretically predicted cjeSvalues. 2 39 Fig. 19. Values of the k 3 / k ~ratio (evaluated from the experimental efficiencies of formation of the excited state in acetonitrile solutions) as a function of the exothermicity of formation AG3 of the localy excited triplet. ADMA, BDMA, FDMA, and PDMA are the A-D compounds with structures presented in Fig. 16. Other A-D system abbreviations denote 4(Panthryl) derivatives of N,N-diethylaniline (ADEA), N,N-di-n-butylaniline (ADBA), N,Ndimethyl-1 -naphthlamine (ADMN), N-methylindoline (AMI),jullolidine (AJ),N,N,3-trismethylaniline (ADMT), and N,N,3,5-tetramethylaniline (ATMA).

Examples of the intramolecular donor-acceptor system: aryl derivatives of N,N-dimethylaniline. PDMA, 4NDMA, 4 4 1-naphthy1)-N,N-dimethylaniline;FDMA, 4-(3-fluoranthyl)-N,N-dimethylaniline; (1-pyreny1)-dirnethylaniline; BDMA 4-(9-acridynyl)-N,N-dirnethylaniline;ADMA, 4-(9-anthryl)-N,Ndimethylaniline. manifold (with the excitation localized on the lowest locally excited triplet of the acceptor or donor subunit). If A and D are large aromatic subunits, the intramolecular electron transfer is associated with the flattening of the molecule in the excited state [68].

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Advances in Electrochemical Science and Engineering, Volume 5 by Richard C. Alkire, Charles W. Tobias

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